Immobilization of ZnO Suspension on Glass Substrate to Remove Filtration During the Removal of Remazol Red R from Aqueous Solution
DOI:
https://doi.org/10.24297/jac.v12i6.6990Keywords:
ZnO film, RRR, Adsorption, Photodegradation, SonicationAbstract
Photodegradation of textile dyes in the presence of an aqueous suspension of semiconductor oxides has been of growing interest. Although this method of destruction of dyes is efficient, the main obstacle of applying this technique in the industry is the time and cost involving separation of oxides from an aqueous suspension. In this research, an attempted was made to develop ZnO films on a glass substrate by simple immobilization method for the adsorption and photodegradation of a typical dye, Remazol Red R (RRR) from aqueous solution. Adsorption and photodegradation of RRR were performed in the presence of glass supported ZnO film. Photodegradation of the dye was carried out by varying different parameters such as the catalyst dosage, initial concentrations of RRR, and light sources. The percentage of adsorption as well as photodegradation increased with the amount of ZnO, reaches a maximum and then decreased. Maximum degradation has been found under solar light irradiation as compared to UV-light irradiation. Removal efficiency was also found to be influenced by the pre-sonication of ZnO suspension.
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References
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[31] Epling G.A. and Lin C., (2002). Photoassisted Bleaching of Dyes Utilizing ZnO and Visible Light. Chemosphere, 46,561-570.
[32] Nasr C., Vinodgopal K., Fisher L., Hotchandani S., Chattopadhyay A. K., and Kamat P. V., (1996). Environmental Photochemistry on Semiconductor Surfaces. Visible Light Induced Degradation of a Textile Diazo Dye, Naphthol Blue Black, on TiO2 Nanoparticles. Journal of Physical Chemistry, 100 (20), 8436-8442.
[2] Anouzla, A., Abrouki, Y., Souabi, S., Safi, M. and Rhbal, H., (2009). Colour and COD Removal of Disperse Dye Solution by a Novel Coagulant: Application of Statistical Design for the Optimization and Regression Analysis. Journal of Hazardous Materials, 166, 1302–1306.
[3] Aksu, Z. and Çağatay, Ş. Ş., (2006). Investigation of Biosorption of Gemazol Turquise Blue-G Reactive Dye by Dried Rhizopus Arrhizus in Batch and Continuous Systems. Separation and Purification Technology, 48 (1), 24-35.
[4] Mahony, O’, T., Guibal, E. and Tobin, J. M., (2002). Reactive Dye Biosorption by Rhizopus Arrhizus Biomass. Enzyme and Microbial Technology, 31 (4), 456-463.
[5] Safa, Y. and Bhatti, H. N., (2011). Biosorption of Direct Red-31 and Direct Orange-26 Dyes by Rice Husk: Application of Factorial Design Analysis. Chemical Engineering Research and Design, 89, 2566–2574.
[6] Fuhs, G. W., and Chen, M., (1975). Microbiological Basis of Phosphate Removal in the Activated Sludge Process for the Treatment of Wastewater. Microbial Ecology, 2, 119-138.
[7] Rajkumar, D., Song, B. J. and Kim, J. G., (2007). Electrochemical Degradation of Reactive Blue 19 in Chloride Medium for the Treatment of Textile Dyeing Wastewater with Identification of Intermediate Compounds. Dyes and Pigments, 72 (1), 1–7.
[8] Pelegrini, R., Peralta-Zamora, P., de Andrade, A. R., Reyes, J. and Durán, N., (1999). Electrochemically Assisted Photocatalytic Degradation of Reactive Dyes. Applied Catalysis B: Environmental, 22 (2), 83–90.
[9] Bódalo-Santoyo, A., Gómez-Carrasco, J.L., Gómez-Gómez, E., Máximo-MartÃn, F. and Hidalgo-Montesinos, A.M., (2003). Application of Reverse Osmosis to Reduce Pollutants Present in Industrial Wastewater. Desalination, 155 (2), 101-108.
[10] Lee, J. M., Kim, M. S., Hwang, B., Bae, W. and Kim, B. W., (2003). Photodegradation of Acid Red 114 Dissolved Using a Photo-Fenton Process with TiO2. Dyes and Pigments, 56, 59–67.
[11] Neamtu, M., Siminiceanu, I., Yediler, A. and Kettrup, A., (2002). Kinetics of Decolorization and Mineralization of Reactive Azo Dyes in Aqueous Solution by the UV/H2O2 Oxidation. Dyes and Pigments, 53 (2), 93–99.
[12] Saquib, M. and Muneer, M., (2002). Semiconductor Mediated Photocatalysed Degradation of an Anthraquinone Dye, Remazol Brilliant Blue R Under Sunlight and Artificial light source. Dyes and Pigments, 53 (3), 237–249.
[13] Robertson, P.K.J., (1996). Semiconductor Photocatalysis: An Environmentally Acceptable Alternative Production Technique and Effluent Treatment Process. J. Cleaner Production, 4 (3-4), 203-212.
[14] Shan, F.K. and Yu, Y.S., (2004). Band Gap Energy of Pure and Al-doped ZnO Thin Films. Journal of the European Ceramic Society, 24 (6), 1869–1872.
[15] Mills, A. and Le Hunte, S. (1997). An Overview of Semiconductor Photocatalysis. Journal of Photochemistry and Photobiology A: Chemistry, 108, 1-35.
[16] Vidal, A., Dinya, Z., Mogyorodi Jr., F. and Mogyorodi, F., (1999 ). Photocatalytic of Thiocarbamate Herbicide Active Ingredients in Water. Applied Catalyst B: Environmental, 21 (4), 259–267.
[17] Sakthivel, S., Neppolian, B., Shankar, M. V., Arabindoo, B., Palanichamy, M. and Murugesan, V., (2003). Solar Photocatalytic Degradation of Azo Dye: Comparison of Photocatalytic Efficiency of ZnO and TiO2. Solar Energy Materials and Solar Cells, 77 (1), 65–82.
[18] Lizama, C., Freer, J., Baeza, J. and Mansilla, H. D., (2002). Optimized Photodegradation of Reactive Blue 19 on TiO2 and ZnO Suspensions. Catalysis Today, 76 (2–4), 235–246.
[19] Kormann, C., Bahnemann, D. W. and Hoffmann, M. R., (1988). Photocatalytic Production of Hydrogen Peroxides and Organic Peroxides in Aqueous Suspensions of Titanium Dioxide, Zinc Oxide, and Desert Sand. Environmental Science & Technology, 22 (7), 798-806.
[20] Chamjangali, M. A. and Boroumand, S., (2013). Synthesis of Flower-like Ag-ZnO Nanostructure and Its Application in the Photodegradation of Methyl Orange. Journal of the Brazilian Chemical Society, 24 (8), 1329-1338.
[21] Apollo, S., Moyo, S., Mabuoa, G. and Aoyi, O., (2014). Solar Photodegradation of Methyl Orange and Phenol Using Silica Supported ZnO Catalyst. International Journal of Innovation, Management and Technology, 5 (3), 203-206.
[22] Zhang, F., Zhao, J., Shen, T., Hidaka, H., Pelizzetti, E., and Serpone, N., (1998). TiO2-Assisted Photodegradation of Dye Pollutants II. Adsorption and Degradation Kinetics of Eosin in TiO2 Dispersions Under Visible Light Irradiation. Applied Catalysis B: Environmental, 15, 147-156.
[23] Hall, D. B., Underhill, P. and Torkelson, J. M., (1998). Spin Coating of Thin and Ultrathin Polymer Films. Polymer Engineering and Science, 38 (12), 2039-2045.
[24] Yao, I. C., Tseng, T. Y. and Lin, P., (2012). ZnO Nanorods Grown on Polymer Substrates as UV Photodetectors. Sensors and Actuators A: Physical, 178, 26–31.
[25] Shah, M. P., Patel, K. A., Nair, S. S., Darji, A. M. and Maharaul, S.,(2013). Microbial Degradation of Azo Dye by Pseudomonas spp. MPS-2 by an Application of Sequential Microaerophilic & Aerobic Process. American Journal of Microbiological Research, 1 (4), 105-112.
[26] Tan, L. K., Kumar, M. K., An, W. W. and Gao, H., (2010). Transparent, Well-Aligned TiO2 Nanotube Arrays with Controllable Dimensions on Glass Substrates for Photocatalytic Applications. Applied Materials and Interfaces, 2 (2), 498–503.
[27] Kemell, M., Pore, V., Tupala, J., Ritala, M. and Leskela, M., (2007). Atomic Layer Deposition of Nanostructured TiO2 Photocatalysts via Template Approach. Chemistry of Materials, 19 (7), 1816-1820.
[28] Zhuang, H. F., Lin, C. J., Lai, Y. K., Sun, L. and Li, J., (2007). Some Critical Structure Factors of Titanium Oxide Nanotube Array in Its Photocatalytic Activity. Environmental Science & Technology, 41, 4735-4740.
[29] Tseng R. L., Wu F. C. and Juang R. S., (2010). Characteristics and Applications of the Lagergren’s First-order Equation for Adsorption Kinetics. Journal of the Taiwan Institute of Chemical Engineers, 41, 661–669.
[30] Fytianos K., Voudrias E. and Kokkalis E., (2000). Sorption-Desorption Behaviour of 2,4-Dichlorophenol by Marine Sediments. Chemosphere, 40 (1), 3-6.
[31] Epling G.A. and Lin C., (2002). Photoassisted Bleaching of Dyes Utilizing ZnO and Visible Light. Chemosphere, 46,561-570.
[32] Nasr C., Vinodgopal K., Fisher L., Hotchandani S., Chattopadhyay A. K., and Kamat P. V., (1996). Environmental Photochemistry on Semiconductor Surfaces. Visible Light Induced Degradation of a Textile Diazo Dye, Naphthol Blue Black, on TiO2 Nanoparticles. Journal of Physical Chemistry, 100 (20), 8436-8442.
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Published
2016-06-16
How to Cite
Kayes, N., Miah, J., Obaidullah, M., Hossain, A., & Hossain, M. (2016). Immobilization of ZnO Suspension on Glass Substrate to Remove Filtration During the Removal of Remazol Red R from Aqueous Solution. JOURNAL OF ADVANCES IN CHEMISTRY, 12(6), 4127–4133. https://doi.org/10.24297/jac.v12i6.6990
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